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- W2075151569 abstract "The decomposition mechanism of photoinduced electron transfer (PET) between electron deficient sensitizers and (phenylazo)triphenylmethane (PAT) was investigated. In 9,10-dicyanoanthracene (DCA) sensitized reaction, benzene, triphenylmethane, 3,3,3-triphenylpropionitrile, and [4-(diphenylmethyl)phenyl]acetonitrile were obtained, and the product distribution was the same as for the direct photolysis and the thermolysis. In the case of 2,4,6-triphenylpyrylium tetrafluoroborate (TPP+) sensitization, the product distribution was drastically changed and 9-phenylfluorene was found to be one of the main products. The results of the irradiation wavelength effects indicate that 9-phenylfluorene is produced by the photoreaction of a trityl cation which is generated by the decomposition of a radical cation of PAT. The results of the experiments of laser flash photolysis suggest that the rate of back electron transfer between a radical anion of the sensitizer and a trityl cation plays an important role in these react..." @default.
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- W2075151569 date "1996-11-01" @default.
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- W2075151569 title "Photoinduced Electron-Transfer Reaction of (Phenylazo)triphenylmethane (PAT). Behavior of Generated Trityl Cation" @default.
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- W2075151569 doi "https://doi.org/10.1246/bcsj.69.3325" @default.
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