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- W2075540004 abstract "The oxidation states of tin, antimony and tellurium isotopes formed predominently (>91%) by fission were investigated in aqueous solutions of 233U irradiated in a reactor. Results were corrected for the thermal reactions with the bulk radiolysis products using tracers for each element. In 0.4 M H2SO4 solutions containing 4.3 mM 233UO22+, 1.5 mM Te(IV) and 1.5 mM Te(VI), the fraction of Te(IV) is 98 ± 2% in the absence of oxygen and 92 ± 3% in the presence of oxygen. In frozen solutions of the same composition, the fraction of Te(IV) is 83 ± 2% in the absence of oxygen and 81 ± 3% in the presence of oxygen. Similar differences are also found in the case of the antimony isotopes in 0.4 M H2SO4 solutions and the tin isotopes in 1 M HCl solutions. For the interpretation of the differences, the reducing action of the species diffusing from the track of the fission fragments are considered." @default.
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- W2075540004 date "1971-12-01" @default.
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- W2075540004 title "A comparison of nuclear charge distribution in thermal-neutron induced fission of 233U and 235U" @default.
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- W2075540004 doi "https://doi.org/10.1016/0022-1902(71)80536-5" @default.
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