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• W2075853506 abstract "We synthesized xKTiO2F–(1−x)BaTiO3 solid solution by the high pressure and temperature method. With regard to the temperature dependence of the dielectric permittivity, the three anomalies corresponding to the three phase transitions of BaTiO3 merged with the increase in x, and only one peak was observed for 0.12≤x≤0.20. The variation in TC with the composition, dTC/dx, of xKTiO2F–(1−x)BaTiO3 was approximately −14 K/mol % for x≥0.12, which is almost the same as and larger than that of the 1/3xBaLiF3−(1−1/3x)BaTiO3 and Ba(Ti1−xMx)O3 (B=Zr, Sn, Hf, and Ce) solid solutions, respectively. This result indicates that the phase transition temperature is significantly affected by the substitution with F ion. Furthermore, it was found that the 0.15KTiO2F−0.85BaTiO3 is an ideal relaxor and that the remnant polarization is 5.6 μC/cm2 at 70 K, which is comparable to that of Ba(Ti0.7Zr0.3)O3. However, the εm of 0.15KTiO2F−0.85BaTiO3 (≈5000 at 100 kHz) was smaller than that of the B-site ion-substituted relaxors: Ba(Ti0.7Zr0.3)O3 and Ba(Ti0.82Sn0.18)O3. Since the remnant polarization of 0.15KTiO2F−0.85BaTiO3 at 70 K was comparable to that of Ba(Ti0.7Zr0.3)O3 at 175 K, the small εm of 0.15KTiO2F−0.85BaTiO3 is found to be due to the decrease in the dielectric permittivity in the paraelectric region." @default.
• W2075853506 created "2016-06-24" @default.
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• W2075853506 date "2008-08-15" @default.
• W2075853506 modified "2023-09-26" @default.
• W2075853506 title "Structure and dielectric properties of high-pressure perovskite-type oxyfluorides xKTiO2F–(1−x)BaTiO3" @default.
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• W2075853506 doi "https://doi.org/10.1063/1.2968246" @default.
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