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• W2076021965 abstract "Off-lattice molecular dynamics simulations are carried out to study fully charged polyelectrolyte brushes with salt, and a comparison with an off-lattice self-consistent field (SCF) theory including finite stretching and volume effects [Biesheuvel et al. Macromolecules 2008, 41, 6254] is presented. The SCF approach is able to reproduce the brush heights at different grafting densities, salt concentrations, and chain lengths on a semiquantitative level. At high grafting densities, the density profiles obtained with both techniques exhibit a particularly close agreement, while at low densities systematic deviations between their shapes are observed. The approximation of local electroneutrality, which the SCF approach is based on, is studied, and its implications are discussed. In this context, the strengths and limitations of the SCF model are analyzed in detail." @default.
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• W2076021965 date "2010-08-16" @default.
• W2076021965 modified "2023-10-18" @default.
• W2076021965 title "Polyelectrolyte Brushes: MD Simulation and SCF Theory" @default.
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• W2076021965 doi "https://doi.org/10.1021/ma101230v" @default.
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