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• W2076163344 endingPage "445401" @default.
• W2076163344 startingPage "445401" @default.
• W2076163344 abstract "We have carried out Ce L- and Mn K-edge x-ray absorption near edge structure (XANES) measurements to experimentally determine the oxidation states of both Ce and Mn in (Sr(1 - x)Ce(x))MnO(3) (x = 0.1-0.4). It was found that although Ce is predominantly 4 + at low doping levels (x = 0.1 and 0.15), the Ce valency decreases with increasing Ce doping (reaching a value of around 3.5 + at x = 0.4). The average Mn oxidation state decreases with the increase of Ce content, with the percentage of Jahn-Teller active Mn(3+) ions increasing from 26% (x = 0.1) to 57% (x = 0.4). Precise structural parameters were also obtained from high resolution neutron diffraction studies for samples with x = 0.1-0.3. The crystal structure remains tetragonal in I4/mcm for x ≤ 0.3. The octahedral tilt angle increases with increasing Ce content, but the distortion of the MnO(6) octahedra is reduced significantly at x ≥ 0.2 due to a transition from long-range ordered Jahn-Teller distortions to incoherent static distortions." @default.
• W2076163344 created "2016-06-24" @default.
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• W2076163344 date "2010-10-10" @default.
• W2076163344 modified "2023-09-24" @default.
• W2076163344 title "X-ray absorption and neutron diffraction studies of (Sr_{1 −<i>x</i>}Ce_<i>x</i>)MnO₃: transition from coherent to incoherent static Jahn–Teller distortions" @default.
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• W2076163344 doi "https://doi.org/10.1088/0953-8984/22/44/445401" @default.
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• W2076163344 hasPublicationYear "2010" @default.
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