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• W2076220247 abstract "Time-resolved Raman scattering measurements were performed on ammonium perchlorate (AP) single crystals under stepwise shock loading. For particular temperature and pressure conditions, the intensity of the Raman spectra in shocked AP decayed exponentially with time. This decay is attributed to shock-induced chemical decomposition in AP. A series of shock experiments, reaching peak stresses from 10−18 GPa, demonstrated that higher stresses inhibit decomposition while higher temperatures promote it. No orientation dependence was found when AP crystals were shocked normal to the (210) and (001) crystallographic planes. VISAR (velocity interferometer system for any reflector) particle velocity measurements and time-resolved optical extinction measurements carried out to verify these observations are consistent with the Raman data. The combined kinetic and spectroscopic results are consistent with a proton-transfer reaction as the first decomposition step in shocked AP." @default.
• W2076220247 created "2016-06-24" @default.
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• W2076220247 creator A5021838658 @default.
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• W2076220247 date "2008-03-21" @default.
• W2076220247 modified "2023-09-27" @default.
• W2076220247 title "Spectroscopic Study of Shock-Induced Decomposition in Ammonium Perchlorate Single Crystals" @default.
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• W2076220247 doi "https://doi.org/10.1021/jp711872u" @default.
• W2076220247 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/18355063" @default.
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