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• W2076243379 abstract "Abstract A new defect-based model for the growth of the fullerene molecule, C60, assembling from a hot, homogenous and dense ensemble of carbon atoms, or “primeval soup”, is presented. Routes comprising swift open channels to fullerene pass through a succession of carbon clusters which are characterised by “magic” numbers related to high reactivity and maximization of the number of dangling bonds per cluster. There is a critical high temperature nucleation leap into three dimensions at the corranulene kernel C20. This is determined by the appearance of a pentagon-based defect, the wedge disclination, which is then in turn responsible for the growth of C60, multiple (or “hedge-hog”) disclinations, higher order fullerenes, nested (and seeded) onion-like clusters and, ultimately, tiny crystalline stable polyhedra. Disclinations play a role in the development of three-dimensional aromatic molecules similar to that of screw dislocations in crystal growth." @default.
• W2076243379 created "2016-06-24" @default.
• W2076243379 creator A5005285003 @default.
• W2076243379 creator A5091449941 @default.
• W2076243379 date "1996-10-01" @default.
• W2076243379 modified "2023-10-06" @default.
• W2076243379 title "Fullerene genesis by ion beams II: Disclinations and the corranulene road" @default.
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• W2076243379 doi "https://doi.org/10.1016/0168-583x(96)00329-1" @default.
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