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• W2076375086 abstract "The general mechanism of the hydroformylation reaction of olefins catalyzed by cobalt and rhodium complexes has been discussed. Particular steps of hydroformylation were studied in a model reaction of hexene-1 with CO/H2 = 1:1 under mild conditions, catalyzed by the Rh(I) complex of the formula Rh(acac)P2 (II) where acac = acetylacetone; P = P(OPh)3. Formation of the following intermediates: Rh(acac)(CO)2P2 (VII), Rh(acac)H2P2 (VIII) and HRh(acac)(CO)P2 (IX) has been confirmed by 1H and 31P NMR and IR methods. Interaction of the hydride species IX with olefin and alkyl complex (X) formation were postulated to be the slowest reactions in the system. The Rh(acac)P2 complex has been found to be a very convenient homogeneous catalyst for mechanistic studies of oxo-reactions under mild conditions." @default.
• W2076375086 created "2016-06-24" @default.
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• W2076375086 date "1983-04-01" @default.
• W2076375086 modified "2023-10-17" @default.
• W2076375086 title "Mechanistic studies on the rhodium complex catalyzed hydroformylation reaction of olefins" @default.
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• W2076375086 doi "https://doi.org/10.1016/0304-5102(83)80019-4" @default.
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