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- W2076407197 abstract "In order to investigate the correlation between electrical transport properties and the transferred exchange interaction between Ni2+ and La3+ in La2NiO4+δ, bulk conductivities and dielectric properties of La2NiO4.02 and La2NiO4.125 have been measured as a function of temperature up to 300 K. The complex-plane impedance analyses determined bulk conductivities. Temperature dependencies of bulk conductivities, the self-consistent agreement of the energies obtained in the bulk conduction and dielectric relaxation processes, and the electron transferred integrals determined in dielectric measurements are indicative of the nonadiabatic hopping conduction, although the conductivity in La2NiO4.125 is very high with a very low hopping energy in comparison with La2NiO4.02. These results have been discussed in terms of the transferred exchange interaction between Ni2+3dz2 orbital and La3+6s orbital through 2pz orbital of apical O2−. With increasing the content of excess oxygen, the decrease in the number of Ni2+3dz2 orbitals, which play an important role in the transferred exchange interaction, changes remarkably the conduction behaviour in La2NiO4.125 from La2NiO4.02." @default.
- W2076407197 created "2016-06-24" @default.
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- W2076407197 date "1999-10-01" @default.
- W2076407197 modified "2023-10-14" @default.
- W2076407197 title "Correlation between hopping conduction and transferred exchange interaction in La2NiO4+ below 300 K" @default.
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- W2076407197 doi "https://doi.org/10.1016/s0921-4526(99)00184-2" @default.
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