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- W2076452403 abstract "Using a flexible Au bag autoclave and a precision high-pressure liquid chromatography pump to control pressure, the liquid–liquid aqueous solubilities of TCE and PCE were measured as a function of temperature from 294 to 434 K (at constant pressure). The results were used to calculate the partial molal thermodynamic quantities of the organic liquid aqueous dissolution reactions: ΔḠsoln, ΔH̄soln, ΔS̄soln and ΔC̄p soln. Calculated values for these quantities at 298 K for TCE are: ΔḠsoln=11.282 (±0.003) kJ/mol, ΔH̄soln=−3.35 (±0.07) kJ/mol, ΔS̄soln=−49.07 (±0.24) J/mol K, and ΔC̄p soln=385.2 (±3.4) J/mol K. Calculated values for these quantities at 298 K for PCE are: ΔḠsoln=15.80 (±0.04) kJ/mol, ΔH̄soln=−1.79 (±0.58) kJ/mol, ΔS̄soln=−59.00 (±1.96) J/mol K and ΔC̄p soln=354.6 (±8.6) J/mol K. These thermodynamic quantities may be used to calculate the solubility of TCE and PCE at any temperature of interest. In the absence of direct measurements over this temperature range, the Henry's Law constants for TCE and PCE have been estimated using the measured aqueous solubilities and calculated vapor pressures." @default.
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- W2076452403 date "2000-05-01" @default.
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- W2076452403 title "The aqueous solubility of trichloroethene (TCE) and tetrachloroethene (PCE) as a function of temperature" @default.
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- W2076452403 doi "https://doi.org/10.1016/s0883-2927(99)00058-x" @default.
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