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- W2076469462 abstract "The atomistic simulation of charge transfer process for an amorphous Alq3 system is reported. By employing electrostatic potential charges, we calculate site energies and find that the standard deviation of site energy distribution is about twice as large as predicted in previous research. The charge mobility is calculated via the Miller–Abrahams formalism and the master equation approach. We find that the wide site energy distribution governs Poole–Frenkel–type behavior of charge mobility against electric field, while the spatially correlated site energy is not a dominant mechanism of Poole–Frenkel behavior in the range from 2×105 to 1.4×106 V/cm. Also we reveal that randomly meshed connectivities are, in principle, required to account for the Poole–Frenkel mechanism. Charge carriers find a zigzag pathway at low electric field, while they find a straight pathway along electric field when a high electric field is applied. In the space-charge-limited current scheme, the charge-carrier density increases with electric field strength so that the nonlinear behavior of charge mobility is enhanced through the strong charge-carrier density dependence of charge mobility." @default.
- W2076469462 created "2016-06-24" @default.
- W2076469462 creator A5029051940 @default.
- W2076469462 creator A5033780451 @default.
- W2076469462 date "2008-07-21" @default.
- W2076469462 modified "2023-10-03" @default.
- W2076469462 title "Atomistic simulation on charge mobility of amorphous tris(8-hydroxyquinoline) aluminum (Alq3): Origin of Poole–Frenkel–type behavior" @default.
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- W2076469462 doi "https://doi.org/10.1063/1.2949506" @default.
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