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- W2076764416 abstract "Abstract A hybrid bilayer membrane (HBM) has been prepared on a glassy carbon electrode (GCE). The HBM consists of an inner layer of n-hexadecylamine (HDA) covalently attached at the GCE and an out-layer of tetra-(N-hexadecylpyridiniurnyl)porphyrin (TC 16 PyP). The HDA was covalently bounded on the carbon surfaces through its primary amine under cyclic voltammetric potential scans forming a self-assembled monolayer (SAM). The TC 16 PyP forms a second layer on top of the HDA layer due to hydrophobic interaction. The TC 16 PyP/HDA/GCE assembly has been utilized to study ion transport through hybrid bilayer membranes. The ion transport through this porphyrin-terminated HBM has been found to strongly dependent on pH. It allows negatively charged redox ions, Fe(CN) 6 3− , to penetrate at pH 3 ) 6 3+ . However, no faradaic current has been detected at pH >6 with either ions. We believe that electrostatic interaction between the redox ions and the charged membrane is the main reason for this pH dependent ion transport." @default.
- W2076764416 created "2016-06-24" @default.
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- W2076764416 date "2011-01-01" @default.
- W2076764416 modified "2023-09-25" @default.
- W2076764416 title "Ion transport through a porphyrin-terminated hybrid bilayer membrane" @default.
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- W2076764416 doi "https://doi.org/10.1016/j.electacta.2010.10.040" @default.
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