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• W2076834650 startingPage "16330" @default.
• W2076834650 abstract "We report a Rh-catalyzed, regio- and enantioselective intermolecular olefin hydroacylation under mild conditions. Hydroacylations between homoallylic sulfides, containing a substrate-bound directing group, and salicylaldehyde derivatives occur in the presence of a spiro-phosphoramidite ligand, (R)-SIPHOS-PE, to give α-branched ketones in >20:1 selectivity and up to 97% ee. Our conditions are also applicable to the asymmetric intermolecular hydroacylation of 1,2-disubstituted olefins." @default.
• W2076834650 created "2016-06-24" @default.
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• W2076834650 date "2010-10-29" @default.
• W2076834650 modified "2023-10-13" @default.
• W2076834650 title "Regio- and Enantioselective Intermolecular Hydroacylation: Substrate-Directed Addition of Salicylaldehydes to Homoallylic Sulfides" @default.
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• W2076834650 doi "https://doi.org/10.1021/ja107198e" @default.
• W2076834650 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/21033718" @default.
• W2076834650 hasPublicationYear "2010" @default.
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