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• W2076877098 abstract "We report the distribution of magnetic moments of Fe3+ and Co2+ in Co2+-, Ti4+-substituted M-type barium hexaferrite, Ba(Co,Ti)xFe(12−2x)O19, as a function of doping rate, x. The substitution, x, for iron has been varied with x=0, 0.25, 0.50, 0.70 and 0.85. The magnetic moments of Fe3+ and Co2+ were calculated from the combined results of Mössbauer measurements for Fe3+ ions in the sublattices and neutron diffraction data for the total moments of Fe3+ and Co2+. A comparison of the signs of the magnetic moments of Fe3+ and Co2+ ions enabled us to attribute spin directions of the Co2+ ions in the sublattices of the substituted ferrite samples. The spin directions of Co2+ are opposite to those of Fe3+ in the 4f2 and 2b sublattices. They are reversed from the original directions in the 4f1 and 12K sublattices when the value of x⩾0.70. A quantitative analysis shows that Co2+ and Ti4+ ions are preferably substituted into 4f2 and 12K sublattices, respectively. In addition, while the hyperfine field of Fe3+ in the 2b sublattice gives rise to the 2b–4f2 interaction it is the partially substituted Co2+ ions in the 4f1 and 12K sublattices that contribute to the near neighbour 2a–4f1 and 2b–12K types of interaction." @default.
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• W2076877098 date "2000-10-01" @default.
• W2076877098 modified "2023-10-11" @default.
• W2076877098 title "Mössbauer spectroscopic determination of magnetic moments of Fe3+ and Co2+ in substituted barium hexaferrite, Ba(Co,Ti)xFe(12−2x)O19" @default.
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• W2076877098 doi "https://doi.org/10.1016/s0304-8853(00)00458-3" @default.
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