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- W2076896716 abstract "Characterization of the pore structures of ferrierite, ZSM—5 and ZSM—11 was performed by measuring the rates and extents of adsorption of a series of molecules of different kinetic diameters. The results were consistent with the reported pore dimensions of the three zeolites. Comparison of activities and selectivities in methanol conversion revealed a direct correlation between the nature of the intracrystalline pore structure and the aromatic product distribution. In addition, a marked enhancement in p-xylene selectivity was observed for mixed ferrierite/ZSM—5 catalysts. Results obtained during but-1-ene isomerization were consistent with an acid-catalysed mechanism involving the secondary butyl carbenium ion as reaction intermediate. A significant feature of but-1-ene isomerization over ferrierite was the marked preferential formation of cis-but-2-ene as reaction product. This was attributed to restricted rotation of the secondary butyl carbenium ion within the constrained environment of the ferrierite pore structure (that is, as a consequence of transition-state selectivity)." @default.
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- W2076896716 date "1987-01-01" @default.
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- W2076896716 title "Comparison of the shape selective properties of ferrierite, ZSM—5 and ZSM—11" @default.
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- W2076896716 doi "https://doi.org/10.1016/0144-2449(87)90114-x" @default.
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