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- W2076944802 abstract "Abstract Vapor-liquid equilibrium measurements have been made for a binary system of ethylene oxide and nonylphenol at four temperatures in the range 363–463 K. At the elevated temperature of interest, the reaction rate of this binary system is too great for conventional measurement techniques to be used. Consequently, a modified adiabatic calorimeter was employed. Use of the calorimeter allows rapid mixing and equilibration of the two components, as well as automated data acquisition. The capability of the calorimeter to collect valid vapor-liquid equilibrium data was established using a nonreactive binary system of pentane and heptane. Data collected at 463 K were compared to predicted values using three different modeling approaches: the Wilson activity coefficient model with the assumption of ideal vapor, the Wilson activity coefficient model combined with the Poynting correction and a modified Redlich-Kwong-Soave equation of state for the vapor phase, and a modified Redlich-Kwong-Soave equation of state for both liquid and vapor phases. Two adjustable parameters were used in each case. Parameters were obtained from the data taken at 363–403 K, where the reaction is slow enough to utilize conventional measurement techniques. The equation of state method gives the best predictions at the higher temperature." @default.
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- W2076944802 date "1993-02-01" @default.
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- W2076944802 title "Measurement and prediction of vapor-liquid equilibria for a reactive system: application to ethylene oxide + nonyl phenol" @default.
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- W2076944802 doi "https://doi.org/10.1016/0378-3812(93)87131-j" @default.
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