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- W2076990930 abstract "Chemical behavior of nitrogen species in intense radiation fields was studied. Simulation models and a N/H/O reaction scheme were developed and verified with a series of experiments. The following results and suggestions were obtained: 1. Ammonium formation rates in water pressurized with H2 and N2 gases at temperatures of 288~473 K were measured and numerically simulated with the reaction scheme within an error factor of 2. 2. Chemical behaviors of radioactive nitrogen (13N and 16N) were also theoretically analyzed. Computer simulations demonstrated that the major species of radioactive nitrogen released to the main steam was nitric oxide (NO). This prediction was partly supported by a 13N analysis in the main steam of an actual BWR: About 85% of the 13N was found to be in anionic species whose precursor was supposed to be NO. 3. Calculated results showed that 13N and 16N in the main steam under hydrogen water chemistry increased similarly but quantitatively not identical with each other: Nitrogen-13 see..." @default.
- W2076990930 created "2016-06-24" @default.
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- W2076990930 date "1991-01-01" @default.
- W2076990930 modified "2023-09-24" @default.
- W2076990930 title "Radiation chemistry of radioactive nitrogen species in BWR reactor cores." @default.
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- W2076990930 doi "https://doi.org/10.3327/jnst.28.347" @default.
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