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• W2076991736 startingPage "1518" @default.
• W2076991736 abstract "We simultaneously measure conductance and force across nanoscale junctions. A new, two-dimensional histogram technique is introduced to statistically extract bond rupture forces from a large data set of individual junction elongation traces. For the case of Au point contacts, we find a rupture force of 1.4 ± 0.2 nN, which is in good agreement with previous measurements. We then study systematic trends for single gold metal-molecule-metal junctions for a series of molecules terminated with amine and pyridine linkers. For all molecules studied, single molecule junctions rupture at the Au-N bond. Selective binding of the linker group allows us to correlate the N-Au bond-rupture force to the molecular backbone. We find that the rupture force ranges from 0.8 nN for 4,4' bipyridine to 0.5 nN in 1,4 diaminobenzene. These experimental results are in excellent quantitative agreement with density functional theory based adiabatic molecular junction elongation and rupture calculations." @default.
• W2076991736 created "2016-06-24" @default.
• W2076991736 creator A5046045254 @default.
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• W2076991736 date "2011-03-02" @default.
• W2076991736 modified "2023-10-17" @default.
• W2076991736 title "Mechanics and Chemistry: Single Molecule Bond Rupture Forces Correlate with Molecular Backbone Structure" @default.
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• W2076991736 doi "https://doi.org/10.1021/nl1042903" @default.
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• W2076991736 hasPublicationYear "2011" @default.
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