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- W2077121294 abstract "Rotational transitions of Al35Cl, Al37Cl, Al79Br, Al81Br, and AlI have been measured in the millimeter wave region. To our knowledge, this is the initial microwave investigation of AlBr and AlI, and for AlI is the first report of any rotational constants. Transitions in excited vibrational states have been measured (up to v=14 for AlI), allowing accurate experimental determination of rotation—vibration interaction terms Y11, Y21, Y31, and Y12 of the Dunham theory. Data analysis yields: for Al35Cl, Be=7313.206(4) MHz, De=7.503(4) kHz, re=2.13011 Å; for Al37Cl, Be=7141.131 (4) MHz, De=7.154(4) kHz, re=2.13011 Å; for Al79Br, Be=4772.825(2) MHz, De=3.3832(11) kHz, re=2.29480 Å; for Al81Br, Be=4742.799(2) MHz, De=3.3408(11) kHz, re=2.29480 Å; and for AlI, Be=3528.5533(8) MHz, De=1.9550(3) kHz, re=2.53709 Å. From nuclear quadrupole couplings the ionic character of the AlI bond is found to be 85%; that of AlBr is found to be ≥87%. From the ionic character of the aluminum monohalides, the electronegativity value of monovalent aluminum is found to be 1.3." @default.
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- W2077121294 date "1972-03-01" @default.
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- W2077121294 title "Millimeter Wave Rotational Spectra of AlCl, AlBr, and AlI" @default.
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- W2077121294 doi "https://doi.org/10.1063/1.1677509" @default.
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