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- W2077222461 abstract "The decomposition probabilities, rate constants, and frequency factors for some olefins have been calculated on the basis of mass spectrometric data and the quasi-equilibrium theory. The rate constant of the parent ion in a homologous series increases with the size of the ion. Fragment ions of the same form but from different parent ions sometimes reveal different rate constants. The scheme of hydrogen molecule abstraction in the secondary decomposition processes of propane is analogous to that of propylene, and reasonable ionic structures of primary ions can be presumed. For a more quantitative discussion, however, there remain some indistinct points in the application of the quasi-equilibrium theory. For instance, the time of reaction along with the rate constant is assumed to be 1×10−5 sec. and to be constant for all ions. Further studies should be carried out both in theory and experiments." @default.
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- W2077222461 date "1962-11-01" @default.
- W2077222461 modified "2023-10-16" @default.
- W2077222461 title "Study on Unimolecular Decomposition of Excited Olefin Ions" @default.
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- W2077222461 doi "https://doi.org/10.1246/bcsj.35.1845" @default.
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