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- W2077382015 abstract "The second- and fourth-order spin-lattice coefficients of ${mathrm{Gd}}^{3+}$ in cubic positions of Th${mathrm{O}}_{2}$ and Ce${mathrm{O}}_{2}$ crystals have been measured as a function of temperature between 4 and 360 ifmmode^circelsetextdegreefi{}K by electron-paramagnetic-resonance experiments in uniaxially stressed crystals. The second-order coefficients are considerably different for the two crystals, and these coefficients show a large variation with temperature. A detailed theoretical calculation of these coefficients has not been carried out; however, it is possible to qualitatively interpret the observed temperature variation in terms of effects due to the modulation of the orbit-lattice interaction by the lattice vibrations. The temperature-variation curves are explained using an Einstein model for the vibrations of the oxygen ligands of the paramagnetic ions. The fourth-order coefficients are similar for the two crystals and are temperature independent in the range studied. The effect of a hydrostatic strain on the energy levels of the ion is used to explain the observed temperature variation of the cubic field parameter in terms of the thermal expansion of the crystal." @default.
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- W2077382015 date "1972-04-01" @default.
- W2077382015 modified "2023-09-23" @default.
- W2077382015 title "Temperature Dependence of the Spin-Lattice Interaction forGd3+in ThO2and CeO2" @default.
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- W2077382015 doi "https://doi.org/10.1103/physrevb.5.2474" @default.
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