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• W2077445483 abstract "The dynamics of solvent reorganization following charge transfer at the interface between two immiscible liquids, one polar and the other non-polar are investigated by molecular dynamics. Both charge separation and charge recombination processes in two different orientations at the surface are considered and are compared with the same processes in the bulk polar solvent. The relaxation at the surface is significantly slower than in the bulk, in contrast to predictions of continuum models. The linear response approximation works reasonably well in the bulk but fails at the interface. The Langevin model is in poor agreement with the exact equilibrium correlations, especially at short time, but can qualitatively account for the overall rate." @default.
• W2077445483 created "2016-06-24" @default.
• W2077445483 creator A5026408688 @default.
• W2077445483 date "1994-03-01" @default.
• W2077445483 modified "2023-10-17" @default.
• W2077445483 title "Solvent dynamics following charge transfer at the liquid-liquid interface" @default.
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• W2077445483 doi "https://doi.org/10.1016/0301-0104(93)e0418-u" @default.
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