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• W2077482330 abstract "We investigate inelastic electron tunneling spectroscopy (IETS) for alkanethiol self-assembled monolayers (SAM) with a scanning tunneling microscope and compare it to first-principles calculations. Using a combination of partial deuteration of the molecule and high-resolution measurements, we identify and differentiate between methyl (CH3) and methylene (CH2) groups and their symmetric and asymmetric C-H stretch modes. The calculations agree quantitatively with the measured IETS in producing the weight of the symmetric and asymmetric C-H stretch modes while the methylene stretch mode is largely underestimated. We further show that inelastic intermolecular scattering is important in the SAM by plotting the theoretical current densities." @default.
• W2077482330 created "2016-06-24" @default.
• W2077482330 creator A5003544621 @default.
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• W2077482330 date "2010-02-18" @default.
• W2077482330 modified "2023-10-03" @default.
• W2077482330 title "Inelastic Tunneling Spectroscopy of Alkanethiol Molecules: High-Resolution Spectroscopy and Theoretical Simulations" @default.
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• W2077482330 doi "https://doi.org/10.1103/physrevlett.104.077801" @default.
• W2077482330 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/20366914" @default.
• W2077482330 hasPublicationYear "2010" @default.
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