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• W2077524818 abstract "In the literature, the electric modulus representation has been used to provide comparative analysis of the ion transport properties in different ion-conducting materials. In this paper we show that the modulus representation is not a suitable tool for such purposes. Our arguments derive from an examination of the scaling properties of both the ac conductivity ${ensuremath{sigma}}^{*}(ensuremath{nu})$ and the modulus ${M}^{*}(ensuremath{nu})$ which demonstrates how scaling that is inherent in ${ensuremath{sigma}}^{*}(ensuremath{nu})$ is lost in ${M}^{*}(ensuremath{nu})$ by inclusion of the high frequency permittivity ${ensuremath{varepsilon}}^{ensuremath{'}}(ensuremath{infty}),$ the latter quantity being unrelated to ion transport processes. Furthermore, we show how highly regarded shape changes of the modulus that occur with varying ion concentration are merely a manifestation of including ${ensuremath{varepsilon}}^{ensuremath{'}}(ensuremath{infty})$ in the definition of ${M}^{*}(ensuremath{nu}).$ We conclude then that the electric modulus formalism has resulted in misleading interpretations of the ion dynamics and, hence, should be discouraged." @default.
• W2077524818 created "2016-06-24" @default.
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• W2077524818 date "2000-12-11" @default.
• W2077524818 modified "2023-10-16" @default.
• W2077524818 title "Ionic conduction in solids: Comparing conductivity and modulus representations with regard to scaling properties" @default.
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• W2077524818 doi "https://doi.org/10.1103/physrevb.63.024301" @default.
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