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• W2077564167 abstract "A first-principles-derived method is used to study the morphology and electric-field-induced evolution of stripe nanodomains in (001) $mathrm{Ba}mathrm{Ti}{mathrm{O}}_{3}$ (BTO) ultrathin films, and to compare them with those in (001) $mathrm{Pb}(mathrm{Zr},mathrm{Ti}){mathrm{O}}_{3}$ (PZT) ultrathin films. The $mathrm{Ba}mathrm{Ti}{mathrm{O}}_{3}$ systems exhibit 180ifmmode^circelsetextdegreefi{} periodic stripe domains at null electric field, as in PZT ultrathin films. However, the stripes alternate along [1--10] in BTO systems versus [010] in PZT systems, and no in-plane surface dipoles occur in BTO ultrathin films (unlike in PZT materials). Moreover, the evolution of the 180ifmmode^circelsetextdegreefi{} stripe domains in the $mathrm{Ba}mathrm{Ti}{mathrm{O}}_{3}$ systems, when applying and increasing an electric field along [001], involves four regions: region I for which the magnitude of the ``down'' dipoles (i.e., those that are antiparallel to the electric field) is reduced, while the domain walls do not move; region II in which some local down dipoles adjacent to domain walls switch their direction, resulting in zigzagged domain walls---with the overall stripe periodicity being unchanged; region III in which nanobubbles are created, then contract along [110] and finally collapse; and region IV which is associated with a single monodomain. Such evolution differs from that of PZT ultrathin films for which neither region I nor zigzagged domain walls exist, and for which the bubbles contract along [100]. Discussion about such differences is provided." @default.
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• W2077564167 date "2007-02-08" @default.
• W2077564167 modified "2023-09-26" @default.
• W2077564167 title "Domain evolution of<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:mi mathvariant=normal>Ba</mml:mi><mml:mi mathvariant=normal>Ti</mml:mi><mml:msub><mml:mi mathvariant=normal>O</mml:mi><mml:mn>3</mml:mn></mml:msub></mml:mrow></mml:math>ultrathin films under an electric field: A first-principles study" @default.
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• W2077564167 doi "https://doi.org/10.1103/physrevb.75.085412" @default.
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