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• W2077777812 abstract "In our investigations of the photoluminescence in poly-(para-phenylene)-type ladder-polymer films a highly nonlinear dependence of the emission spectra is observable at elevated excitation densities. A spectral redistribution results in the hyperlinear increase of emission efficiency in the blue region, as the vibronic 0-1 transition $(ensuremath{lambda}=492mathrm{nm})$ becomes the most predominant radiative relaxation. The detailed study of temporal decay and spectral evolution of luminescence provided by streak camera measurements performed in the temperature range $T=20--300mathrm{K}$ reveals the spectrum being composed by the contributions of two different emitting species, namely, ${S}_{1}$-singlet states and aggregates. The material is found to be photochemically stable and luminescence does not seem to be limited by saturation effects even under high-excitation conditions, which is essential for laser application." @default.
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• W2077777812 date "1997-07-15" @default.
• W2077777812 modified "2023-09-23" @default.
• W2077777812 title "Picosecond spectroscopy and hyperlinear photoluminescence in poly(para-phenylene)-type ladder polymers" @default.
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• W2077777812 doi "https://doi.org/10.1103/physrevb.56.1632" @default.
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