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• W2077889119 endingPage "417" @default.
• W2077889119 startingPage "408" @default.
• W2077889119 abstract "The spectral substructure and the dynamics of the OH- and OD-stretching bands of HDO in the diluted isotopic mixtures with D2O and for the first time H2O are investigated using 2-color IR spectroscopy with tunable subpicosecond pulses. From the observed transient band shapes, we derive four major spectral components within the OH-band of HDO in the solvent D2O peaked at approximately 3330 cm-1 (I), 3390 cm-1(II), 3460 cm-1 (III), and 3520 cm-1 (IV), as well as three corresponding species in the case of the OD-band in the solvent H2O. The components display no distinct temperature dependence of position and spectral width in the investigated temperature range 273−343 K. Comparing the OH-stretching mode of HDO:D2O to the OD-vibration of HDO:H2O, the population lifetime increases significantly from 1.0 ps for OH to 1.8 ps (±0.2 ps) for OD at room temperature, whereas spectral relaxation, assigned to structural changes, seems to slow from 1.0 ± 0.4 ps to 2.0 ± 0.8 ps in the protonated water environment." @default.
• W2077889119 created "2016-06-24" @default.
• W2077889119 creator A5015460416 @default.
• W2077889119 creator A5037050218 @default.
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• W2077889119 date "2001-12-15" @default.
• W2077889119 modified "2023-09-27" @default.
• W2077889119 title "Subpicosecond Spectroscopy of Liquid Water in the Infrared: Effect of Deuteration on the Structural and Vibrational Dynamics" @default.
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• W2077889119 doi "https://doi.org/10.1021/jp011047p" @default.
• W2077889119 hasPublicationYear "2001" @default.
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