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• W2077892135 abstract "The influence of an external uniform electrostatic field on the internal energy and polarization of a medium-sized water cluster, consisting of 40 molecules is studied at four temperatures: 150, 170, 200, and 240 K, by means of the Monte Carlo method. The external field is slowly varied in the 0.5×107–7×107 V/cm range. The system shows an abrupt change of its properties at some critical value of the field, Etr, where a transition from a normal (solid-like or liquid-like) to a superpolarized cluster state is observed. This process has the character of a first-order phase transition and is accompanied by the absorption of heat. For intermediate field strengths, polarization has been found to increase with increasing temperature, an effect, which through a simple analytical model has been shown to be the result of the interplay between the strength of the attractive water–water interactions and the strength of the external field. Also Etr has been found to decrease with increasing temperature, in contrast to the behavior dictated by the Clausius–Clayperon equation for field-induced transitions between equilibrium states." @default.
• W2077892135 created "2016-06-24" @default.
• W2077892135 creator A5030316386 @default.
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• W2077892135 date "2002-09-01" @default.
• W2077892135 modified "2023-10-01" @default.
• W2077892135 title "Electric field induced transitions in water clusters" @default.
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• W2077892135 doi "https://doi.org/10.1016/s0166-1280(02)00111-2" @default.
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