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- W2077972890 abstract "Es werden potentiostatische Einschaltversuche an glatten Platinkathoden in HNO3/HNO2-Mischungen wechselnder Konzentration geschildert. Die Versuche ermöglichen einen nahezu quantitativen Vergleich zwischen der Kinetik der kathodischen Reduktion der Salpetersäure zu salpetriger Säure und der chemischen Kinetik der salpetrigen Säure nach Abel und H. Schmid. Aus den Einschaltoszillogrammen ergeben sich im Rahmen der Versuchsfehler die Geschwindigkeitskonstanten, die nach der Abel-Schmidschen Kinetik zu erwarten sind. Form und Lage der Oszillogramme werden auf Grund des folgenden Mechanismus berechnet: Single transient experiments under potentiostatic conditions at smooth platinum electrodes in HNO3/HNO2-mixtures of various composition are described. The experiments make it possible to compare almost quantitatively the kinetics of the cathodic reduction of nitric to nitrous acid with the chemical kinetics of nitrous acid according to Abel and H. Schmid. From the oscillographs rate constants are obtained within the limits of experimental error as are to be expected according to the kinetics of Abel and Schmid. Shape and position of the oscillograms were calculated on the basis of the following mechanism:" @default.
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- W2077972890 date "1964-09-01" @default.
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- W2077972890 title "Die autokatalytische Natur der kathodischen Reduktion von Salpetersäure zu salpetriger Säure IV. Der potentiostatische Einschaltvorgang [1]" @default.
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- W2077972890 doi "https://doi.org/10.1002/bbpc.19640680714" @default.
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