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- W2078166795 abstract "Abstract Porous cryptomelane-type octahedral molecular sieve manganese oxide (K-OMS-2) supported iron nanocatalysts have been developed for selective hydrogenation of CO 2 and CO to light olefins. Surface coated iron (SCI) catalysts and frame-work doped iron (FDI) catalysts have different interfaces. The synergistic interactions of nano-size iron carbides, potassium promoters, and manganese oxides vary in these two types of the Fischer-Tropsch (F-T) catalysts with respect to their catalytic activities and selectivity. For example, the SCI catalysts have high selectivity (>95%) to light olefins but low catalytic activity with a CO conversion of 45% and a CO 2 conversion of 32%. The FDI catalysts showed higher catalytic activities with a CO conversion of 87% and a CO 2 conversion of 45%. Direct analyses in real time-mass spectra and temperature programmed reduction-mass spectra have been used to correlate temperature effects. These component–structure–activity relationships provide insight for CO 2 utilization and F-T syntheses." @default.
- W2078166795 created "2016-06-24" @default.
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- W2078166795 date "2013-03-01" @default.
- W2078166795 modified "2023-10-13" @default.
- W2078166795 title "Selective hydrogenation of CO2 and CO to useful light olefins over octahedral molecular sieve manganese oxide supported iron catalysts" @default.
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- W2078166795 doi "https://doi.org/10.1016/j.apcatb.2012.11.003" @default.
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