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• W2078237750 abstract "Photofragmentation of the uracil molecule following carbon 1s core ionization and the subsequent Auger deacy has been investigated. The applied technique, photoelectron–photoion–photoion coincidence (PEPIPICO) spectroscopy allows simultaneous detection of momentum-correlated photoions together with the photoelectron and makes possible a detailed investigation of different fragmentation processes. In order to help the fragment identification, also uracil where one of the carbon atoms was replaced by 13C was measured, with the assumption that replacement of one C atom by 13C does not alter the fragmentation. An earlier investigation concerning thymine and 5-bromouracil was a strong motivation for the present study. The present results confirm the starting hypothesis for the pattern analysis, that the fragmentation process is preceded by only one starting geometry of the parent molecule, followed by a number of sequential bond cleavages and that all pyrimidine derivatives have very similar fragmentation behavior. However, the replacement of a hydrogen atom by methyl group, i.e., the transition from uracil to thymine, seems to narrow the range of possible ion fragments." @default.
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• W2078237750 date "2011-09-01" @default.
• W2078237750 modified "2023-10-05" @default.
• W2078237750 title "Fragmentation patterns of core ionized uracil" @default.
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• W2078237750 doi "https://doi.org/10.1016/j.ijms.2011.07.006" @default.
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