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• W2078385003 abstract "A membrane reactor that incorporated hollow fiber in combination with an established catalyst was used for the oxidative coupling of methane (OCM). A perovskite membrane of the composition BaCoxFeyZrzO3−δ (BCFZ, x + y + z = 1) allows a controlled oxygen feed into the reactor over its axial length. Using this novel hollow fiber membrane reactor with a 2 wt % Mn/5 wt % Na2WO4 on SiO2 catalyst as a packed bed around the fiber, oxygen separation from air and C2 formation could be established at 800 °C with long-term stability. The highest C2 selectivity of ∼75% was observed at a methane conversion of 6% with a C2H4:C2H6 ratio of 2:1. The highest C2H4:C2H6 ratio of 4:1 and maximum C2 yield of 17% was obtained at 50% C2 selectivity. It is known from the literature that such results can be obtained without a catalyst in a similar membrane reactor only at temperatures 150 °C higher." @default.
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• W2078385003 date "2010-04-08" @default.
• W2078385003 modified "2023-10-18" @default.
• W2078385003 title "Oxidative Coupling of Methane in a BCFZ Perovskite Hollow Fiber Membrane Reactor" @default.
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• W2078385003 doi "https://doi.org/10.1021/ie100282g" @default.
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