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• W2078389743 abstract "Zinc complexes of methyl 31-demethyl-bacteriopheophorbides-d possessing a 2-(un)substituted ethynyl or ethenyl group at the 20-position were prepared through palladium-catalyzed cross-coupling of their 20-bromide with the corresponding alkyne or alkene. The synthetic zinc 20-substituted 3-hydroxymethyl-131-oxo-chlorins self-aggregated in an aqueous micellar solution to give similar large oligomers as self-aggregates of bacteriochlorophylls in the core part of the main light-harvesting antenna of photosynthetic green bacteria. The zinc 20-ethynyl-chlorin fully gave the self-aggregates, but its 202-substitution disturbed the self-aggregation. The 20-(2-phenyl)ethenyl moieties induced the formation of relatively smaller oligomers as well as residual monomers due to their steric bulkiness." @default.
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• W2078389743 date "2014-05-01" @default.
• W2078389743 modified "2023-10-16" @default.
• W2078389743 title "Synthesis of zinc 20-substituted bacteriochlorophyll-d analogs and their self-aggregation" @default.
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• W2078389743 doi "https://doi.org/10.1016/j.tetlet.2014.04.057" @default.
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