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• W2078446739 abstract "The composition of the spinel phase in the system LiMnO is studied under the influence of a controlled gas atmosphere and temperature/time schedule. The existence of an extended spinel phase of composition Li[Mn2 − xLix]O4 − δ (0 ≤ x ≤ 13) is shown. The LiMn ratio as well as the proportion between Mn3+ and Mn4+ is adjustable by the method of preparation. LiMn2O4 − δ can be prepared in a cubic and tetragonal modification. According to magnetic and spectroscopic measurement, no simple ionic model can describe the electron structure throughout the entire series of solid solution. A partial charge delocalization takes place resulting in a reduction of the total number of unpaired electrons. At lower temperatures a spin glass behaviour develops due to the inherent frustration of the octahedral antiferromagnetic sublattice. The freezing temperature depends on the LiMn ratio and decreases with increasing x." @default.
• W2078446739 created "2016-06-24" @default.
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• W2078446739 date "1996-08-02" @default.
• W2078446739 modified "2023-09-25" @default.
• W2078446739 title "Influence of processing on the Li:Mn ratio in spinel phases of the system Li1 + xMn2 − xO4 − δ" @default.
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• W2078446739 doi "https://doi.org/10.1016/0167-2738(96)00349-9" @default.
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