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• W2078451807 abstract "Abstract New mixed‐valence Cu I –Cu II 1D coordination polymers of the structure [Cu I 2 Cu II X 2 (Pip‐dtc) 2 (CH 3 CN) 2 ] n [Pip‐dtc = piperidine‐1‐carbodithioate; X = Br ( 1a ), I ( 1b )] containing a dithiocarbamate derivative have been synthesized and structurally characterized by X‐ray diffraction. The 1D infinite chains were formed from mononuclear copper units [Cu(Pip‐dtc) 2 ] connected by bromido‐ or iodido‐bridged copper dinuclear units that include acetonitrile ligands {i.e., [Cu 2 X 2 (CH 3 CN) 2 ]}. Evaluation of the magnetic properties of 1a and 1b revealed that these complexes displayed relatively strong antiferromagnetic interactions [ J = –20.4 cm –1 ( 1a ) and J = –18.8 cm –1 ( 1b )] between unpaired electrons of the copper(II) ions through the dinuclear halido–copper(I) units. Impedance spectroscopy revealed that complexes 1a and 1b exhibit intriguing semiconducting properties at activation energies of E a = 0.78 eV ( 1a ) and E a = 0.62 eV ( 1b ). Coordination polymers 1a and 1b were then adopted as the sensitizing material in dye‐sensitized solar cells (DSSCs)." @default.
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• W2078451807 date "2013-05-15" @default.
• W2078451807 modified "2023-10-18" @default.
• W2078451807 title "Halido‐Bridged 1D Mixed‐Valence Cu ^I –Cu ^II Coordination Polymers Bearing a Piperidine‐1‐carbodithioato Ligand: Crystal Structure, Magnetic and Conductive Properties, and Application in Dye‐Sensitized Solar Cells" @default.
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• W2078451807 doi "https://doi.org/10.1002/ejic.201300188" @default.
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