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• W2078473428 abstract "Vibrational (v) state-selected reaction probabilities (PvjJ) have been calculated for the reaction He+H2+(v=0,1,2,3)→HeH++H, for H2+ in its ground rotational state (j=0) for a range of total angular momentum (J) values, for total energy (E) in the range 0.94–1.4 eV, using time-dependent quantum mechanical (TDQM) approach and centrifugal sudden approximation. The number of oscillations in Pv0J(E) decreases with increase in J. In addition, there is a noticeable increase in the threshold energy (Eth) with increase in J. The magnitude of Pv0J decreases with increase in J resulting in converged cross section values by the time J becomes 35–45, depending upon v and E under investigation. The resulting (converged) reaction cross section values are in excellent agreement with the experimental results at E=1.14 eV, both in terms of the magnitude and in terms of the observed vibrational enhancement. Interestingly, there is a noticeable discrepancy between our TDQM results and earlier time-independent quantum mechanical studies at higher energies, for v=1 and 2. For v=3, the difference between the two theoretical studies is the largest near the threshold. Our results for v=2 and 3 suggest that the oscillations in the vibrational state-selected reaction cross section values are amenable to experimental observation." @default.
• W2078473428 created "2016-06-24" @default.
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• W2078473428 date "2002-11-12" @default.
• W2078473428 modified "2023-10-11" @default.
• W2078473428 title "Reaction probabilities and reaction cross sections for three-dimensional He+H2+(v) collisions: A time-dependent quantum mechanical study" @default.
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• W2078473428 doi "https://doi.org/10.1063/1.1518002" @default.
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