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• W2078520140 abstract "Carbon has unfaired advantages in material properties to be used as electrodes. It offers a low cost, light weight cathode that minimizes the loss in specific energy of lithium–oxygen batteries as well. To date, however, carbon dioxide evolution has been an unavoidable event during the operation of non-aqueous lithium–oxygen batteries with carbon electrodes, due to the reactivity of carbon against self-decomposition and catalytic decomposition of electrolyte. Here we report a simple but potent approach to eliminate carbon dioxide evolution by using an ionic solvate of dimethoxyethane and lithium nitrate. We show that the solvate leads to deactivation of the carbon against parasitic reactions by electrochemical doping of nitrogen into carbon. This work demonstrates that one could take full advantage of carbon by mitigating the undesired activity. Carbon dioxide evolution during the charging process in lithium–oxygen batteries is generally both unavoidable and undesirable. Here, Kang et al. use an ionic solvate of dimethoxyethane and lithium nitrate to deactivate the carbon electrode, which completely eliminates the evolution of carbon dioxide." @default.
• W2078520140 created "2016-06-24" @default.
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• W2078520140 date "2014-05-22" @default.
• W2078520140 modified "2023-10-13" @default.
• W2078520140 title "Deactivation of carbon electrode for elimination of carbon dioxide evolution from rechargeable lithium–oxygen cells" @default.
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• W2078520140 doi "https://doi.org/10.1038/ncomms4937" @default.
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• W2078520140 hasPublicationYear "2014" @default.
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