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• W2078632368 abstract "We investigated the spectral feature and fluorescence lifetime of quasimonolayered porphyrins at very short distance to metal substrates (1–2.5nm) through fine-tuning the length of alkanethiols. The ordered self-assembled monolayers of alkanethiols on Au(111) act as a uniform electronic decoupling layer and suppress the interface quenching via charge transfer. However, the fluorescence quenching via nonradiative energy transfer to the metal still prevails in the porphyrin-alkanethiol-metal sandwich structures. The decay rates are found to follow a 1∕d3 dependency on spacer thickness, which suggests that the classical electromagnetic theory appears still valid at distance down to 1nm through volume damping." @default.
• W2078632368 created "2016-06-24" @default.
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• W2078632368 date "2008-06-02" @default.
• W2078632368 modified "2023-10-15" @default.
• W2078632368 title "Fluorescence decay of quasimonolayered porphyrins near a metal surface separated by short-chain alkanethiols" @default.
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• W2078632368 doi "https://doi.org/10.1063/1.2938861" @default.
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