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• W2078679971 abstract "We engineered specific microfluidic devices based on the pervaporation of water through a PDMS membrane, to formulate continuous and steady concentration gradients of a binary aqueous molecular mixture at the nanolitre scale. In the case of a model complex fluid (a triblock copolymer solution), we demonstrate that such a steady gradient crosses the phase diagram from pure water up to a succession of highly viscous mesophases. We then performed in situ spatially resolved measurements (confocal spectroscopy and small-angle X-ray scattering) to quantitatively measure the concentration profile and to determine the microstructure of the different textures. Within a single microfluidic channel, we thus screen quantitatively and continuously the phase diagram of a complex fluid. Beside, as such a gradient corresponds to an out-of-equilibrium regime, we also extract from the concentration measurement a precise estimate of the collective diffusion coefficient of the mixture as a function of the concentration. In the present case of the triblock copolymer, this transport coefficient features discontinuities at some phase boundaries, which have never been observed before." @default.
• W2078679971 created "2016-06-24" @default.
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• W2078679971 date "2013-01-01" @default.
• W2078679971 modified "2023-09-25" @default.
• W2078679971 title "Steady and out-of-equilibrium phase diagram of a complex fluid at the nanolitre scale: combining microevaporation, confocal Raman imaging and small angle X-ray scattering" @default.
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• W2078679971 doi "https://doi.org/10.1039/c2lc41207a" @default.
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