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- W2078683116 abstract "The photodissociation spectra of size‐selected Ca+(H2O)n (n=1–6) ions are examined in the wavelength region from 330 to 1440 nm by monitoring the total yield of the fragment ions. The absorption bands exhibit redshifts as large as ∼16 000 cm−1 with respect to the 2P–2S resonance line of the free Ca+ ion and are explained by the shift of this transition as a result of hydration. The converging trend in the spectral shifts at n∼6 is discussed in relation to the filling of the first solvation shell for Ca+ undergoing the sdσ hybridization. We also discuss the possible contribution of charge‐transfer character in the observed transitions in conjunction with our recent results on the photoelectron spectra of Na−(NH3)n. The mass spectra of the fragment ions show the existence of two dissociation channels: The evaporation of water molecules and the dehydrogenation reaction to produce the hydrated CaOH+ ions. The evaporation process is the dominant decay channel for n=1, while the reaction is the only one for n≥3..." @default.
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- W2078683116 date "1996-06-22" @default.
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- W2078683116 title "Photodissociation study on Ca<sup>+</sup>(H<sub>2</sub>O)<sub><i>n</i></sub>, <i>n</i>=1–6: Electron structure and photoinduced dehydrogenation reaction" @default.
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- W2078683116 doi "https://doi.org/10.1063/1.471738" @default.
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