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• W2078986237 startingPage "6351" @default.
• W2078986237 abstract "We report here on the motional and fluorescence lifetime dynamics of the chromophore NBDHA (6-(N-(7-nitrobenz-2-oxa-1,3-diazol-4-yl)amino)hexanoic acid) in neat solvents and in aqueous solutions containing unilamellar vesicles of varying composition. We measure the transient response of this chromophore by time-correlated single-photon counting, using one- and two-photon excitation to resolve the Cartesian components of the rotational diffusion constant, D. Our experimental data for NBDHA in selected solvents of varying viscosity demonstrate that one- and two-photon excitation probe different components of the rotational diffusion constant and that this chromophore reorients as a prolate rotor with an aspect ratio of ∼2. For NBDHA in aqueous solutions containing unilamellar vesicles of varying composition, we recover the same reorientation behavior regardless of vesicle composition. Fluorescence lifetime and steady-state fluorescence data show the chromophore to reside in a polar environment that is different from neat water. We understand these data in the context of the chromophore residing in close proximity to the unilamellar vesicle polar headgroups in all cases." @default.
• W2078986237 created "2016-06-24" @default.
• W2078986237 creator A5002615133 @default.
• W2078986237 creator A5090602198 @default.
• W2078986237 date "2006-03-01" @default.
• W2078986237 modified "2023-09-25" @default.
• W2078986237 title "Quantitating the Dynamics of NBD Hexanoic Acid in Homogeneous Solution and in Solutions Containing Unilamellar Vesicles" @default.
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• W2078986237 doi "https://doi.org/10.1021/jp057073v" @default.
• W2078986237 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/16553453" @default.
• W2078986237 hasPublicationYear "2006" @default.
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