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• W2078995104 abstract "We report a study of hydrogen storage and its mechanism in a novel material, representing single-walled carbon nanotubes (SWCNTs) encapsulated by thin Pd layers onto a Pd substrate. A synergetic effect resulting in combination of the Pd and the SWCNT properties with regard to hydrogen has been achieved. We showed that adding SWCNTs increases the H2-capacity of the Pd–SWCNT composite under electrochemical loading only by up to 25% relative to the Pd metal alone. At the same time, with regard to the added SWCNTs, such synergetic approach (providing high H2 pressure from highly H-loaded massive Pd substrate into a small fraction of deposited SWCNT) allowed us to achieve a net capacity of 8–12 wt.%. H2, thus, bringing a unique chance to study hydrogen storage mechanism in highly H-loaded SWCNT. Using ESR technique it was established that the Pd–Cx π-complexes forming at the openings of SWCNTs could be considered as hydrogen adsorption sites, providing both high gravimetric capacity (H/C > 1) and low hydrogen binding energy in the Pd encapsulated SWCNT." @default.
• W2078995104 created "2016-06-24" @default.
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• W2078995104 date "2009-05-01" @default.
• W2078995104 modified "2023-09-24" @default.
• W2078995104 title "Evidence for large hydrogen capacity in single-walled carbon nanotubes encapsulated by thin Pd layers onto a Pd substrate" @default.
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• W2078995104 doi "https://doi.org/10.1016/j.diamond.2008.11.029" @default.
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