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- W2079043178 abstract "This paper describes the thermodynamics and kinetics of the corrosion of U[sub x]Zr[sub 1-x]C[sub 1-y] in hydrogen gas. It describes how corrosion rates are influenced by variables such as pressure, temperature, and gas flow rate. A model is developed which agrees with experimental steady-state corrosion rates at 1 atm between 2670 and 3100 K. It is shown that under steady-state conditions the corrosion flux is rate limited by the vapor phase transport of Zr(g) away from the solid surface to the bulk gas stream where the partial pressure of Zr(g) is determined by the congruently vaporizing surface composition. Extrapolation of the model to higher pressures indicates that Zr(g) transport should also be rate limiting at higher pressures but the corrosion rate should decrease slightly with increased hydrogen pressure due to reduced gaseous diffusion rates. The model predicts that the corrosion rate will increase as the square root of gas velocity for a given temperature and pressure. Calculations demonstrating the effects of gas velocity are in agreement with experimental studies." @default.
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- W2079043178 date "1993-01-01" @default.
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- W2079043178 title "A thermokinetic model describing the vaporization behavior of U{sub x}Zr{sub 1-x}C{sub 1-y} in hydrogen" @default.
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