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- W2079062634 abstract "A probability theory has been developed to account for the effects of sequential collisional excitation in collisional-activation mass spectrometry. With simplifying assumptions concerning the collisional-activation mechanisms, cross-sections and the collisional energy-transfer probability Pc(E), expressions have been derived for the parent-ion and total daughter-ion intensities in collisional-activation spectra. One of the indications of the theory is that when sequential collisional excitation becomes appreciable, the usual Beer's law expression for precursor-ion attenuation holds only approximately. Also, it has been shown that some information concerning Pc(E) may be obtained from collisional-activation experiments. Applying the expressions to collisional-activation data for 8.0 keV methane molecular ions, the parent-ion and total daughter-ion intensities can be accounted for adequately using the present theory. Also, it appears that the effects of sequential collisional excitation are significant." @default.
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- W2079062634 date "1983-05-01" @default.
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- W2079062634 title "Fragmentation probability in collisional-activation mass spectrometry (CA/MS). I. Effects of sequential collisional excitation" @default.
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- W2079062634 doi "https://doi.org/10.1016/0020-7381(83)80009-6" @default.
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