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• W2079073921 abstract "Through photolysis of NF3/HI/M=1.5/0.5/38 Torr mixtures (M=N2,CO,Ar) in a grating cavity, HF rotational laser emission is produced for (v=0, J=21→20), (1,23→22), (2,24→23), and (3,18→17). Known attenuators are placed in the laser cavity and used to estimate the absolute population inversions responsible for the laser gains. The results confirm the role of selective V→R resonant pumping of these high J rotational lasers. Further, they provide rough estimates for the Δv=2, Δ J=10, and Δv=3, Δ J=20 near-resonant V→R rate constants for HF relaxation by N2 from v=4, J=14, and v=5, J=3, 4, and 5 to v=2, J=24. These estimates fall in the range 10−13 to 10−14 cm3/molecule s, indicating that for N2 collision partners, HF multiquantum processes with Δv=3 may contribute a few percent of the total v=5 vibrational relaxation rate. They also suggest that, for both N2 and CO, V→R near-resonant channels (including Δv=1) provide the dominant relaxation process." @default.
• W2079073921 created "2016-06-24" @default.
• W2079073921 creator A5056470238 @default.
• W2079073921 creator A5057035718 @default.
• W2079073921 date "1984-08-01" @default.
• W2079073921 modified "2023-10-18" @default.
• W2079073921 title "HF multiquantum V→R relaxation rates with N2 and CO" @default.
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• W2079073921 doi "https://doi.org/10.1063/1.447767" @default.
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