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- W2079147531 abstract "Total reflection X-ray absorption fine structure (TR-XAFS) has been utilized for the detailed analyses of the surface aggregation of double-tailed quaternary ammonium ion bromides. TR-XAFS at the Br K-edge gives us information on the population of Br− just below the subphase surface as well as its local structure. The spectra indicate that Br− is almost completely hydrated, even when it is attracted by the compressed monolayer. In addition, the signal intensities obtained for the monolayers of the ammonium amphiphiles with different hydrocarbon chain lengths suggest that the correction for the attenuation of X-rays due to the absorption by the hydrocarbon layer is necessary to obtain a reliable population of Br− on the subphase surface. The correction of the attenuation reveals that the population of Br− is lower than that predicted on the basis of the electrostatic attraction, and that this deviation becomes larger as the monolayer is compressed. These findings can be explained by the submergence of Br− ..." @default.
- W2079147531 created "2016-06-24" @default.
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- W2079147531 date "2009-06-23" @default.
- W2079147531 modified "2023-09-23" @default.
- W2079147531 title "Evacuation of Counteranions from Langmuir Monolayers of Double-Tailed Quaternary Ammonium Ions into Subphase at High Surface Pressures as Studied by Total Reflection X-ray Absorption Spectrometry" @default.
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- W2079147531 doi "https://doi.org/10.1021/jp900912z" @default.
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