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• W2079245369 abstract "Next‐generation micro‐solid oxide fuel cells for portable devices require nanocrystalline thin‐film electrolytes in order to allow fuel cell fabrication on chips at a low operation temperature and with high power outputs. In this study, nanocrystalline gadolinia‐doped ceria (Ce 0.8 Gd 0.2 O 1.9− x ) thin‐film electrolytes are fabricated and their electrical conductivity and thermodynamic stability are evaluated with respect to microstructure. Nanocrystalline gadolinia‐doped ceria thin‐film material (Ce 0.8 Gd 0.2 O 1.9− x ) exhibits a larger amount of defects due to strain in the film than state‐of‐the‐art microcrystalline bulk material. This strain in the film decreases the ionic conductivity of this ionic O 2− conductor. The thermodynamic stability of a nanocrystalline ceria solid solution with 65 nm grain size is reduced compared with microcrystalline material with 3–5 μm grain size. Nanocrystalline spray‐pyrolyzed and PLD Ce 0.8 Gd 0.2 O 1.9− x thin films with average grain sizes larger than 70 nm show predominantly ionic conductivity for temperatures lower than 700°C, which is high enough to be potentially used as electrolytes in low to intermediate‐temperature micro‐solid oxide fuel cells." @default.
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• W2079245369 date "2007-06-01" @default.
• W2079245369 modified "2023-10-18" @default.
• W2079245369 title "Thermodynamic Stability of Gadolinia-Doped Ceria Thin Film Electrolytes for Micro-Solid Oxide Fuel Cells" @default.
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• W2079245369 doi "https://doi.org/10.1111/j.1551-2916.2007.01531.x" @default.
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