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- W2079261019 abstract "The objective of the present investigation is initiated and designed to determine the kinetic data (activation energy and the pre-exponential factor) for catalytic oxidation of lean premixed preheated hydrogen–air mixtures over non-noble metals (binary mixtures of Co3O4/Cr2O3) and platinum catalysts at atmospheric pressure. A one-dimensional, non-equilibrium, unsteady mathematical model of the catalytic combustion in a packed bed reactor had been developed. The model includes conduction, convective and radiative heat transfer, axial diffusion, and accounts for both homogeneous and heterogeneous reactions of the Arrhenius type. Numerical simulation had been conducted for a range of equivalence ratios, superficial velocities, and inlet temperatures for inert and catalytic beds. It had been found that the pre-exponential factor for hydrogen–air mixture is 5·4 × 10−5 kmol m−2 s−1 and the activation energy for platinum catalyst is 10·0±0·5 and 9·4±0·6 kJ mol−1 at inlet temperature below and above 350 K respectively. An activation energy of 10·3±1·0 kJ mol−1 over the Co3O4/Cr2O3 catalyst had been obtained." @default.
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- W2079261019 date "2006-12-01" @default.
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- W2079261019 title "Modelling of hydrogen oxidation within catalytic packed bed reactor" @default.
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- W2079261019 doi "https://doi.org/10.1179/174602206x148874" @default.
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