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- W2079340544 abstract "The increased sensitivity of organic materials to electron beam radiation damage in the presence of ice was demonstrated by using polymer latex spheres embedded in ice as well characterized model systems. Rapid etching of ice occurs at the ice-organic material interface. The damage to the polymer depends on its chemical nature: some, e.g. polystyrene, lose mass by etching and decrease in size, while others such as poly(methylmethacrylate) swell, and lose most of their mass. These phenomena are very different from what one finds in the absence of ice. It is suggested that free-radical reactions that involve chemical species from the ice and the organic material are responsible for these phenomena. Comparison of polycrystalline versus vitreous frozen aqueous solutions of glycerol of about the same composition has shown that the vitreous samples are much more susceptible to radiation damage. This is probably caused by the very intimate contact between water and glycerol molecules in the vitreous state. This gives rise to reactions involving free radicals produced by solvent and solute. Phase segregation upon crystallization limits the free-radical reactions between ice and the organic solute." @default.
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- W2079340544 date "1984-01-01" @default.
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- W2079340544 title "Radiation damage to organic inclusions in ice" @default.
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- W2079340544 doi "https://doi.org/10.1016/0304-3991(84)90098-6" @default.
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