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- W2079352936 abstract "Abstract Ultrafast transient absorption measurement system with cavity-dumped chromium:forsterite (Cr:F) laser as a light source was developed. The second harmonic of the Cr:F laser can cover the immeasurable region of the titanium:sapphire laser which is nowadays the most popular light source for the ultrafast spectroscopy. The second harmonic of the Cr:F laser was tunable from 620 to 640 nm and the shortest pulse duration attained in the present condition was ∼25 fs. The sensitivity of this laser to ultrafast spectroscopy was evaluated by the measurement of S 0 and S 1 state dynamics of azulene. In spite of extremely small molar extinction coefficient of the S 1 ←S 0 transition, i.e. 300 M −1 cm −1 , the ultrafast dynamics of azulene after photo-excitation to S 1 state was clearly observed with high S/N ratio and ≤30 fs time resolution. Although the small molar extinction coefficient value of 300 M −1 cm −1 , pump-and-probe measurement clearly resolved the multi-exponential recovery profile with a very weak oscillation of 160 cm −1 ." @default.
- W2079352936 created "2016-06-24" @default.
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- W2079352936 date "2003-03-01" @default.
- W2079352936 modified "2023-09-26" @default.
- W2079352936 title "Development of kinetic analysis system in pump–probe measurement based on femtosecond chromium: forsterite laser and its application to S1–S0 relaxation dynamics of azulene" @default.
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- W2079352936 doi "https://doi.org/10.1016/s1010-6030(02)00407-0" @default.
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